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Stable isotopic analysis was undertaken for the gunpowder ingredients from crude saltpetre and propellants from several types of gun that prevailed during the late 19th century in south‐western Japan. Stable isotopic signatures for δ15Nsaltpetre nitrogen, δ34Snative sulphur and δ13Ccharcoal carbon in crude saltpetre, gunpowder magazines bearing the trademark of mills from southern Scotland and cartridges for an improved Sharps rifle (with a US trademark) all imply common assemblages from the same source (saltpetre and native sulphur from British India and Sicily, respectively) in the United Kingdom (UK). One Pritchett patron is common for muzzle‐loading Enfield rifles, while the other suggests a four‐allied lead bullet for an unidentified hand gun. Propellants in the Pritchett patron from the same institution also suggest a common source of these rifles. On the contrary, the ingredients for an unidentified rifle and time fuse for a Paixhans gun with unique stylistic devices showed distinctive isotopic signatures, indicating a local Japanese origin. The Pritchett patron from the Kumamoto Museum involved a mixed provenance from the UK and Japan. The stable isotopic analysis provides direct evidence for the ultimate origin of the propellant.  相似文献   
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This study conducted petrographic and geochemical analyses of chert artifacts from the Late Middle Paleolithic, the Initial Upper Paleolithic, the Early Upper Paleolithic, and the Epi-Paleolithic assemblages in the Jebel Qalkha area, southern Jordan, to examine their correlations with the visual attributes and diachronic variability. The results revealed two different aspects of the petrographic and geochemical signatures. The first aspect showed some correlations with the visual chert types that were characterized by the abundance/preservation of fossils, the enrichment of several elements (i.e., Ca, Sr, and Ba), and the quartz crystallite size. The second aspect of geochemical signatures, such as Fe, Mn, Ni, Cr, and Co, showed no correlation with the visual types but was correlated with the chrono-cultural groups. Given the chert occurrences and variability in and around the study area, the first aspect of the chert variability likely represents the variations of different chert outcrops as well as the internal variations within the same sources. Whether the second aspect represents chrono-cultural changes in the use of chert sources needs to be clarified in future by our ongoing examination of geological chert samples in the study area.  相似文献   
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