Ground-based microwave radiometry to determine stratospheric and mesospheric ozone profiles

From April 1984 to April 1985 a microwave radiometer was operated at Bern (Switzerland, latitude 47°N) measuring the thermal emission of the rotational ozone transition at 142.2 GHz to determine stratospheric and mesospheric ozone abundances in the range ~25–~75 km altitude. From a total of 334 retrieved day-time profiles, monthly mean ozone partial pressures for Umkehr layers 6–10 were calculated. On this basis ozone variations compare favorably with Umkehr data from the nearby Arosa (Switzerland, 150 km east of Bern) station and with a monthly zonal mean model compiled from satellite data by Keating and Young. From the microwave data an annual mean ozone distribution was determined. The method retrieves somewhat larger ozone volume mixing ratios between 25 and 30 km altitude. For the rest of the measurement range of the sensor there is good agreement with 20 year annual mean ozone values from Arosa, with the Krueger and Minzner profile and with the respective annual mean data given by Keating and Young. The microwave ozone sensor can easily be adapted for operational use, where it can supplement and expand the measurement range of the traditional Umkehr network.     

1987–1989 total ozone and ozone sounding observations in Northern Scandinavia and Antarctica,and the climatology of the lower stratosphere during 1965–1988 in Northern Finland

The total ozone observations of Tromsö (Northern Norway), Sodankylä (Northern Finland) and Murmansk (Northwestern Soviet Union) for 1987–1989 have been studied. Comparisons of the total ozone with stratospheric temperatures observed at Sodankylä have been made. These values have also been compared with the long-term mean total ozone at Tromsö and the long-term means of stratospheric temperatures at Sodankylä. No severe ozone depletions were observed. The exceptionally high total ozone values at these stations in February 1989 were connected to abnormally high stratospheric temperatures. The comparison of total ozone observed at roughly the same southern latitudes revealed great differences in the springtime.The 1989 ozone sounding observations of Sodankylä, Bear Island and Ny Ålesund (Spitzbergen) did not reveal any indications of pronounced ozone depletion. A comparative study of ozone, temperature and relative humidity indicated that the springtime variability of ozone in the lower stratosphere was clearly connected to meteorological variability. The lower tropospheric ozone had two distinct maxima, one in spring with large-scale photochemical causes and the other in summer connected with the emissions of hydrocarbons and oxides of nitrogen in Europe.Temperature observations made at Sodankylä over 24 yr revealed the existence of a potential for polar stratospheric cloud formation in the lower stratosphere in winter and early spring. A trend analysis of 50 hPa temperature revealed a negative trend of −0.16 K/yr in January and a positive trend of 0.15 K/yr in April; the annually-averaged trend was only −0.02 K/yr for this 24-yr period. When the January–February mean temperatures are separated according to the phase of the QBO in the tropical stratosphere, correlations between temperatures and sunspot numbers are found.     

The middle atmospheric response to short and long term solar UV variations: analysis of observations and 2D model results

We have investigated the middle atmospheric response to the 27-day and 11-yr solar UV flux variations at low to middle latitudes using a two-dimensional photochemical model. The model reproduced most features of the observed 27-day sensitivity and phase lag of the profile ozone response in the upper stratosphere and lower mesosphere, with a maximum sensitivity of +0.51% per 1% change in 205 nm flux. The model also reproduced the observed transition to a negative phase lag above 2 mb, reflecting the increasing importance with height of the solar modulated HO_x chemistry on the ozone response above 45 km. The rnodel revealed the general anti-correlation of ozone and solar UV at 65–75 km, and simulated strong UV responses of water vapor and HO_x species in the mesosphere. Consistent with previous 1D model studies, the observed upper mesospheric positive ozone response averaged over ±40° was simulated only when the model water vapor concentrations above 75 km were significantly reduced relative to current observations. Including the observed temperature-UV response in the model to account for temperature-chemistry feedback improved the model agreement with observations in the middle mesosphere, but did not improve the overall agreement above 75 km or in the stratosphere for all time periods considered. Consistent with the short photochemical time scales in the upper stratosphere, the model computed ozone-UV sensitivity was similar for the 27-day and 11-yr variations in this region. However, unlike the 27-day variation, the model simulation of the 11-yr solar cycle revealed a positive ozone-UV response throughout the mesosphere due to the large depletion of water vapor and reduced HO_x-UV sensitivity. A small negative ozone response at 65–75 km was obtained in the 11-yr simulation when temperature-chemistry feedback was included,In agreement with observations, the model computed a low to middle latitude total ozone phase lag of +3 days and a sensitivity of +0.077% per 1% change in 205 nm flux for the 27-day solar variation, and a total ozone sensitivity of +0.27% for the 11-yr solar cycle. This factor of 3 sensitivity difference is indicative of the photochemical time constant for ozone in the lower stratosphere which is comparable to the 27-day solar rotation period but is much shorter than the 11-yr solar cycle.     

Climatology of the middle atmosphere of the Southern hemisphere

Main features of spatial distribution and time variations of meteorological parameters in the Southern hemisphere at altitudes 25–80 km are reviewed on the basis of zonal empirical models revised in 1982. Meridional distribution and seasonal variations are analysed. For comparison purposes with the Northern hemisphere, a model developed by Cole and Kantor in 1978 is used. It is revealed that the compilation of new models of the Southern hemisphere atmosphere has not resulted in substantial revision of hemispheric-structure outlined earlier in studies conducted in the Central Aerological Observatory. Meridional distribution of the parameters in summer is characterized by higher values of temperature, pressure and density gradients in the stratosphere of the Southern hemisphere than in that of the Northern hemisphere. This resulted in greater advancement of the core of the summer-time easterly (low towards the equator in the Southern hemisphere than in its northern counterpart. In winter, meridional temperature gradients in the middle stratosphere are greater in the Southern hemisphere than those in the Northern hemisphere, however, rapid attenuation of the gradients with height is observed in the Southern hemisphere, and above 35–40 km they become negative near 50–60°S, in contrast to positive values typical for the Northern hemisphere stratosphere. In the wind field, specific features of the Southern hemisphere westerly flow are high intensity and relatively low altitude of the maximum speed (as compared to the Northern hemisphere).The phases of the annual temperature wave at low latitudes are similar south and north of the equator; south of 30°S a reversal of the phase is observed. The semi-annual oscillation of temperature and wind is less pronounced in middle and high latitudes of the Southern hemisphere than in the Northern hemisphere.The origin of the primary differences between the hemispheres is related mainly to lower intensity of large-scale stratospheric processes in the Southern hemisphere as compared to those in the Northern hemisphere, which is confirmed by values of the standard deviation of the parameters in the two hemispheres.In summer, temperature and pressure fields based on satellite data are symmetric relative to the poles in both hemispheres. In winter, the distortion of the mean pressure field in the mesosphere may be as great in the Southern as in the Northern hemisphere.     

Large scale coherence of the mesospheric and upper stratospheric temperature fluctuations

A large set of temperature profiles has been obtained in the upper stratosphere and the mesosphere over Europe during the MAP/WINE compaign by the use of different techniques: datasondes and falling spheres launched by metrockets, ground-based OH spectrometers and a Rayleigh lidar. These data have been used to study the large scale variability of the middle atmosphere during the winter 1983–1984. The temperature variations with periods longer than 25 days are clearly related to the succession of minor upper stratospheric warmings observed during this winter. The variations in the period range 10–20 days are at least partially due to westward propagating Rossby waves, of which one mode, with a 12.5 days period, is tentatively identified as the second symmetric mode of the wave number 2.     

Stratospheric warmings and their effects on the winds in the upper atmosphere during the winter of MAP/WINE 1983–1984

A comparison is made between winds near 95 km altitude obtained from meteor radar measurements at Sheffield and radiances for the top channel of a stratospheric sounding unit (SSU). Three minor warmings and a major warming in the stratosphere during the period 25 December 1983 to 4 March 1984 were found to be associated with characteristic changes in both the zonal and meridional components of the wind above the mesopause. Similar systematic variations in the winds were observed around 12 December 1983, suggesting that a minor warming, the first of the season, developed at that time in the stratosphere. This event has not previously been reported. Its occurrence is confirmed by radiances from the SSU.     

Modelling of ozone reduction by stratospheric aircraft

Using a two-dimensional model of the atmospheric circulation and composition, different scenarios of the effects of stratospheric aircraft on ozone layer destruction were calculated. It is shown that the ozone loss depends strongly on the altitude and composition of engine emissions from high-speed civil transport aircraft. The inclusion in the two-dimensional model of the effects of chemical eddies results in significantly reduced ozone losses in the high latitudes of the northern hemisphere during wintertime, when the dynamics of the stratosphere are strongly disturbed by planetary waves. This result can be connected with the increase of stratosphere/troposphere exchange.     

Upper stratospheric and mesospheric temperatures derived from lidar observations at Aberystwyth

From lidar observations of relative atmospheric density above Aberystwyth (52.4°N, 4.1°W) upper stratospheric and mesospheric temperatures have been derived for a total of 93 nights between December 1982 and February 1985. Excellent agreement was found between radiances synthesised from these temperatures and those measured by satellite-borne instruments. Summer temperatures showed a smooth and regular variation with altitude and reasonably good agreement with the CIRA (1972) model atmosphere. By contrast, winter temperatures showed a much greater variability with altitude and greater changes from night to night, with the frequent occurrence of a large amplitude wave-like perturbation in the mesosphere with about 15 km vertical wavelength and amplitude about 20K between 60 and 80 km.Pronounced warmings of the stratosphere were observed during the three winters of observation. During the warming event occurring in early February 1983 the stratopause temperature increased to 303K at 43 km, while the major warming event of late December 1984/early January 1985 produced a stratospheric temperature gradient of 16K km⁻¹ between 34 and 36 km. During the latter event a distinct local temperature minimum at 32.6 km was observed on New Year's Eve, this descending to 29 km by the following night and being accompanied by a lowering of the stratopause from 43 to 38.5 km in the same period. These results demonstrate the ability of the present technique to resolve the high stratopause temperatures and steep stratospheric temperature gradients which occur during stratospheric warmings, in marked contrast to the limited resolution achieved by satellite experiments.     

Dominant vertical scales of gravity waves in the middle atmosphere observed with the MU radar and rocketsondes

We have simultaneously observed wind motions in the altitude range of 5–90 km by means of the MU radar, rocketsondes and radiosondes. Dominant vertical scales of wind fluctuations due to gravity waves were 2–5 km in the lower stratosphere, about 5–15 km in the upper stratosphere and longer than 15 km in the mesosphere. The increase in the vertical scale with altitude is interpreted in terms of the saturation of upward propagating gravity waves. In the stratosphere, the observed vertical wavenumber spectra showed smaller amplitudes and more gradual slopes than the model values. Furthermore, the wind velocity variance in the stratosphere increases exponentially with an e-folding height of about 9 km, implying that the gravity waves were not fully saturated. On the other hand, the spectra in the upper stratosphere and mesosphere agreed fairly well with the model spectra. The variance in the mesosphere seems to cease increase of the wave amplitudes and agrees reasonably well with the model value.     

A study of equatorial waves in the Indian zone

An equatorial wave campaign was conducted at Trivandrum (8.5°N, 77°E), Minicoy (8.3°N, 73°E) and Port Blair (11.7°N, 92.7°E) during June-July 1988. The campaign provided balloon-measured daily wind profiles at all the three stations for 48 days in the 0–30 km altitude range and rocket-measured daily wind profiles at Trivandrum for 42 days in the 31–60 km altitude range. Using these daily wind data a study was made on different equatorial wave modes present in this region. The study revealed evidence of Kelvin waves with period 12–16 days and vertical wavelength ∼ 10 km in the lower stratosphere, with period 6–9.6 days and vertical wavelength of ∼ 10–15 km in the stratospheric-lower mesospheric region and MRG waves with periods 4–4.4 days and vertical wavelength of 10 km in the upper troposphere and lower stratosphere.     

Summertime stratospheric wind measurements above the South Pole

Observations of the mean wind flow and wave motions in the stratosphere at the South Pole are presented. The atmospheric motions are determined from the tracking of a high altitude, zero-pressure balloon launched from Amundsen-Scott Station during the austral summer of 1985–1986. The balloon position was precisely monitored by an optical theodolite for a large portion of the flight so that small scale motions could be resolved. The mean flow above the pole was approximately 3ms⁻¹. Atmospheric motions characteristic of internal gravity waves were observed with an intrinsic period of approximately 4.5 h and vertical and horizontal wavelengths of approximately 2.5km and 125km, respectively. The horizontal perturbation velocity of the observed waves was large compared to the mean horizontal flow velocity. The implication is that wave motions play a dominant role in the transport of stratospheric constituents in regions where the mean winds are light, such as over the South Pole during austral summer.     

Ozone “miniholes” initiated by energetic solar protons

In this study, it is shown that during four Solar Proton Events (SPE), mostly of the Ground Level Event (GLE) type (May 1990, September and October 1989, and March 1989), inside the polar cap in the Arctic (or the Antarctic) short-term depletions were observed (up to 20%) in the ozone total content. These depletions or so-called ozone “miniholes” seem to be caused by energetic solar protons with energies of 150–300 MeV. For May 1990, the gas phase photochemical model includes only 1% ozone depletion compared with 18% observed at Barentsburg (Svalbard), and for none of the other events can homogeneous processes explain the observed depletion. The problem seems to be solved considering heterogeneous reactions in the presence of increased amounts of aerosol particles in the stratosphere which may be triggered by penetrating solar protons, or through an additional decrease of temperature, or through an increase of volume electric charge in the stratosphere (or even troposphere).     

A mid-latitude ground-based lidar study of stratospheric warmings and planetary wave propagation

A survey of stratospheric and mesospheric temperature was performed on a regular basis during winter conditions from the lidar station of the Observatory of Haute Provence (44°N, 6°E). The method uses the range resolved Rayleigh scattering of a laser beam and its latest performances are given. The data presented in this paper cover two winter periods and include the major stratospheric warmings of 1980 and 1981; the results obtained by lidar are compared with global stratospheric data obtained by the radiosonde network and from the SSU satellite experiment. It is shown how the extension of the measurements into the mesosphere (and simultaneously in the stratosphere) and the height resolution achievable with the lidar technique permits one to estimate the time-delay of the downward propagation of a warming from the mesosphere to the low stratosphere in about 20 days. The influence of planetary wave propagation is also shown to produce a periodic variation in the stratopause height even in the absence of the stratospheric warming reported by the STRATALERT messages.     

Tropical behavior of mesospheric ozone as observed by SMM

The seasonal behavior of low latitude mesospheric ozone, as observed by the SMM satellite solar occultation experiment, is detailed for the 1985–1989 period. Annual as well as semi-annual waves are observed in the 50–70 km altitude region. In the latitude range of ±30 the ozone phase and amplitude are functions of temperature and seasonal changes in solar flux. Temperature is the controlling factor for the equatorial region and seasonal changes in solar flux become more dominant at latitudes outside the equatorial zone (greater than ±15). There is a hemispheric asymmetry in the ozone annual wave in the 20 30 region, with northern hemispheric ozone having a larger amplitude than southern hemispheric ozone. In this region temperature is nearly in phase with ozone in both hemispheres and is reduced in amplitude in the northern hemisphere. The equatorial region is characterized by a strong semi-annual wave in addition to the annual variation, and temperature is nearly out of phase with ozone. At all latitudes there is a larger ozone concentration at sunrise than at sunset. The sunrise sunset difference increases with increasing altitude     

Mean winds observed by the Kyoto meteor radar in 1983–1985

Mean winds at 82–106 km altitude have been almost continuously monitored by the Kyoto meteor radar over the period from May 1983 to December 1985. The mean zonal wind becomes eastward with amplitudes as large as 30 m s⁻¹ in the summer months (May–August), maximizing early in July at 95 km altitude, while it is less than 10 m s⁻¹ at all the observed altitudes during the equinoxes. It is normally eastward in winter at low altitudes, although it sometimes becomes westward during sudden stratospheric warmings. The mean meridional wind is usually equatorward and is weaker than the zonal component. A southward wind exceeding 10 m s⁻¹ is detected in July and August. The observed mean winds are compared with the CIRA 1972 model and coincidences with sudden warmings of changes in zonal wind direction are pointed out.     

Long-term tropospheric and lower stratospheric ozone variations from ozonesonde observations

An analysis is presented of the long-term mean pressure latitude seasonal distribution of tropospheric and lower stratospheric ozone for the four seasons covering, in part, over 20 years of ozonesonde data. The observed patterns show minimum ozone mixing ratios in the equatorial and tropical troposphere except in regions where net photochemical production is dominant. In the middle and upper troposphere, and low stratosphere to 50 mb, ozone increases from the tropics to subpolar latitudes of both hemispheres. In mid stratosphere, the ozone mixing ratio is a maximum over the tropics. The observed vertical ozone gradient is small in the troposphere but increases rapidly above the tropopause. The seasonal variation at a typical mid latitude station (Hohenpeissenberg) shows a summer maximum in the low to middle troposphere, shifting to a winter-spring maximum in the upper troposphere and lower stratosphere and spring -summer maximum at 10 mb. The amplitude of the annual variation increases from a minimum in the tropics to a maximum in polar regions. Also, the amplitude increases with height at all latitudes up to about 30 mb where the phase of the annual variation changes abruptly. The phase of the annual variation is during spring in the boundary layer, summer in mid troposphere, and spring in the upper troposphere and lower stratosphere. The annual long-term ozone trends are significantly positive at about + 1.2% yr in mid troposphere (500 mb) and significantly negative at about − 0.6% yr¹ in the lower stratosphere(50mb)     

Poker Flat MST radar observations of high latitude neutral winds at the mesopause during and after solar proton events

Observations with the Poker Flat, Alaska, MST radar during and after solar proton events in 1982 and 1984 suggest that winds in the altitude range of ~ 80–90 km were altered as a consequence of the influx of energetic charged particles and large electric fields at high latitudes. The atmospheric changes accompanying these events appear to result in a reduction of the semidiurnal tide and an enhancement in the diurnal tide. It is suggested that these changes could result from the alteration of the local tidal heating distribution produced by the particle precipitation, either through changes in the local ozone distribution or as a result of mesospheric Joule heating.     

Measurement of O2(a1Δg) emission in a total solar eclipse

The altitude distribution of the oxygen infrared atmospheric bands at 1.27 μm was measured during the total solar eclipse of 26 February 1979. The ozone concentration profile has been derived from these airglow measurements and indicates that at 85 km the concentration at totality was 7 × 1.7 cm⁻³, with no well defined upper layer. This reduced concentration, which is typical of summertime conditions, was probably due to perturbations in the mesospheric chemistry and transport induced by a winter warming event that was in progress at the time of the eclipse. At 60 km the ozone concentration, 2.7 × 10¹⁰ cm⁻³, was enhanced above that normally measured. This increase may also have been caused by the stratospheric warming event but the effects of a particle precipitation event, which was also in progress during the eclipse, may be important.     

Influence of latitudinal and longitudinal variations of ozone and water vapour on the solar semidiurnal tide

A new tidal source model, based on climatological global ozone and water vapour distributions, has been obtained for January, April, July and October. The source model is used for modelling the solar semidiurnal tide in the lower thermosphere within the framework of the classical tidal theory. The observed phase quasibimodality of the semidiurnal tide at middle latitudes is possibly formed, to a great extent, by two types of hemispheric asymmetry (changing sharply near the equinox) of the ozone distribution. Near 95 km at middle latitudes, the ozone and water vapour distribution nonzonality yields typical values ~2 m/s for maximum longitudinal variations of the zonal and meridional wind amplitudes, and the range ~0.2–0.5 h for maximum longitudinal phase variations in the Northern hemisphere, while they can reach ~10 m/s and ~1.5 h in the Southern hemisphere. The hemispheric asymmetry is mainly caused by the effect of the water vapour tidal source.     

The 27 day solar UV response of stratospheric ozone: solar cycle 21 vs. solar cycle 22

A correlative study of ozone and the solar UV flux on the time scale of a solar rotation shows an anomalous response of ozone in the upper stratosphere during solar cycle 22. The study, which is based on the analysis of ozone and solar UV flux measured by the SBUV/2 spectrometer on NOAA 11 (January 1989–December 1990), shows a sharp transition from an in-phase relation between ozone and the solar UV flux below 2 mb to an almost out-of-phase relation above 1 mb. Such a phase change is not predicted by photochemical models and was not observed during solar cycle 21. The ozone measurements from the Nimbus-7 SBUV spectrometer from 1979 to 1984 showed an almost in-phase relation between ozone and the solar UV flux at these heights (in agreement with model predictions). Similar studies of ozone and temperature relations between 30 and 1 mb did not show significant changes from the solar cycle 21 to 22. The temperature oscillations appear to be primarily of dynamical origin, with no apparent correlation with solar UV flux.